Electrochemical Synthesis of Hybrid Layered Thermoelectric Materials Based on PEDOT/SnS Doped with Ag

José F. Serrano-Claumarchirant; Ana María Igual-Muñoz; Mario Culebras; Maurice N. Collins; Andrés Cantarero; Clara M. Gómez

doi:10.1002/admi.202100951

Electrochemical Synthesis of Hybrid Layered Thermoelectric Materials Based on PEDOT/SnS Doped with Ag

José F. Serrano-Claumarchirant, Ana María Igual-Muñoz, Mario Culebras, Maurice N. Collins, Andrés Cantarero, Clara M. Gómez

School of Engineering

Research output: Contribution to journal › Article › peer-review

Abstract

Due to the increasing energy demand and public awareness of climate change and environmental problems, sustainable energy development has become one of the most strategic areas of research. In this work, a hybrid layered thermoelectric material is produced, which consists of the combination of poly(3,4-ethylenedioxythiophene) (PEDOT) and tin sulfide (SnS). The films are produced by the electrochemical deposition of SnS on the surface of a PEDOT electrode. The thermoelectric properties are optimized by controlling the doping level of SnS by adding Ag. As a consequence, the power factor is remarkably improved up to 58.6 µW m^–1 K^–2, which is more than two orders of magnitude higher than that of the undoped materials.

Original language	English
Article number	2100951
Journal	Advanced Materials Interfaces
Volume	8
Issue number	23
DOIs	https://doi.org/10.1002/admi.202100951
Publication status	Published - 8 Dec 2021

Keywords

electrodeposition
flexible materials
hybrid thermoelectrics
PEDOT
tin sulfide

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Access to Document

10.1002/admi.202100951

Cite this

@article{31ec193d31bb401eaab728277fa8ae6b,

title = "Electrochemical Synthesis of Hybrid Layered Thermoelectric Materials Based on PEDOT/SnS Doped with Ag",

abstract = "Due to the increasing energy demand and public awareness of climate change and environmental problems, sustainable energy development has become one of the most strategic areas of research. In this work, a hybrid layered thermoelectric material is produced, which consists of the combination of poly(3,4-ethylenedioxythiophene) (PEDOT) and tin sulfide (SnS). The films are produced by the electrochemical deposition of SnS on the surface of a PEDOT electrode. The thermoelectric properties are optimized by controlling the doping level of SnS by adding Ag. As a consequence, the power factor is remarkably improved up to 58.6 µW m–1 K–2, which is more than two orders of magnitude higher than that of the undoped materials.",

keywords = "electrodeposition, flexible materials, hybrid thermoelectrics, PEDOT, tin sulfide",

author = "Serrano-Claumarchirant, {Jos{\'e} F.} and Igual-Mu{\~n}oz, {Ana Mar{\'i}a} and Mario Culebras and Collins, {Maurice N.} and Andr{\'e}s Cantarero and G{\'o}mez, {Clara M.}",

note = "Publisher Copyright: {\textcopyright} 2021 The Authors. Advanced Materials Interfaces published by Wiley-VCH GmbH.",

year = "2021",

month = dec,

day = "8",

doi = "10.1002/admi.202100951",

language = "English",

volume = "8",

journal = "Advanced Materials Interfaces",

issn = "2196-7350",

number = "23",

}

TY - JOUR

T1 - Electrochemical Synthesis of Hybrid Layered Thermoelectric Materials Based on PEDOT/SnS Doped with Ag

AU - Serrano-Claumarchirant, José F.

AU - Igual-Muñoz, Ana María

AU - Culebras, Mario

AU - Collins, Maurice N.

AU - Cantarero, Andrés

AU - Gómez, Clara M.

PY - 2021/12/8

Y1 - 2021/12/8

N2 - Due to the increasing energy demand and public awareness of climate change and environmental problems, sustainable energy development has become one of the most strategic areas of research. In this work, a hybrid layered thermoelectric material is produced, which consists of the combination of poly(3,4-ethylenedioxythiophene) (PEDOT) and tin sulfide (SnS). The films are produced by the electrochemical deposition of SnS on the surface of a PEDOT electrode. The thermoelectric properties are optimized by controlling the doping level of SnS by adding Ag. As a consequence, the power factor is remarkably improved up to 58.6 µW m–1 K–2, which is more than two orders of magnitude higher than that of the undoped materials.

AB - Due to the increasing energy demand and public awareness of climate change and environmental problems, sustainable energy development has become one of the most strategic areas of research. In this work, a hybrid layered thermoelectric material is produced, which consists of the combination of poly(3,4-ethylenedioxythiophene) (PEDOT) and tin sulfide (SnS). The films are produced by the electrochemical deposition of SnS on the surface of a PEDOT electrode. The thermoelectric properties are optimized by controlling the doping level of SnS by adding Ag. As a consequence, the power factor is remarkably improved up to 58.6 µW m–1 K–2, which is more than two orders of magnitude higher than that of the undoped materials.

KW - electrodeposition

KW - flexible materials

KW - hybrid thermoelectrics

KW - PEDOT

KW - tin sulfide

UR - http://www.scopus.com/inward/record.url?scp=85118850725&partnerID=8YFLogxK

U2 - 10.1002/admi.202100951

DO - 10.1002/admi.202100951

M3 - Article

AN - SCOPUS:85118850725

SN - 2196-7350

VL - 8

JO - Advanced Materials Interfaces

JF - Advanced Materials Interfaces

IS - 23

M1 - 2100951

ER -

Electrochemical Synthesis of Hybrid Layered Thermoelectric Materials Based on PEDOT/SnS Doped with Ag

Abstract

Keywords

UN SDGs

Access to Document

Other files and links

Fingerprint

Cite this