Kinetics of the Selective Catalytic Reduction of no by NH3 Over a Commercial Catalyst

W. R.A.M. Robinson; J. G. van Ommen; A. Woldhuis; J. R.H. Ross

doi:10.1016/S0167-2991(08)64377-3

Kinetics of the Selective Catalytic Reduction of no by NH₃ Over a Commercial Catalyst

W. R.A.M. Robinson
, J. G. van Ommen
, A. Woldhuis
, J. R.H. Ross

Research output: Contribution to journal › Article › peer-review

Abstract

Kinetic measurements were performed on the reduction of NO by NH₃ over a commercial ‘DeNox’ catalyst in order to test several kinetic models. The best results were obtained with a simple Power Rate Law model. Progressively less accurate predictions were given by a modified Eley-Rideal model, a two-site Langmuir-Hinshelwood model, a one-site Langmuir-Hinshelwood model, and finally a ‘pure’ Eley-Rideal model.

Original language	English
Pages (from-to)	2673-2676
Number of pages	4
Journal	Studies in Surface Science and Catalysis
Volume	75
Issue number	C
DOIs	https://doi.org/10.1016/S0167-2991(08)64377-3
Publication status	Published - 1 Jan 1993
Externally published	Yes

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title = "Kinetics of the Selective Catalytic Reduction of no by NH3 Over a Commercial Catalyst",

abstract = "Kinetic measurements were performed on the reduction of NO by NH3 over a commercial {\textquoteleft}DeNox{\textquoteright} catalyst in order to test several kinetic models. The best results were obtained with a simple Power Rate Law model. Progressively less accurate predictions were given by a modified Eley-Rideal model, a two-site Langmuir-Hinshelwood model, a one-site Langmuir-Hinshelwood model, and finally a {\textquoteleft}pure{\textquoteright} Eley-Rideal model.",

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AU - Ross, J. R.H.

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AB - Kinetic measurements were performed on the reduction of NO by NH3 over a commercial ‘DeNox’ catalyst in order to test several kinetic models. The best results were obtained with a simple Power Rate Law model. Progressively less accurate predictions were given by a modified Eley-Rideal model, a two-site Langmuir-Hinshelwood model, a one-site Langmuir-Hinshelwood model, and finally a ‘pure’ Eley-Rideal model.

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Kinetics of the Selective Catalytic Reduction of no by NH₃ Over a Commercial Catalyst

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